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Critical stages of the brewing process for changes in antioxidant activity, color and flavor.
HELEN WOFFENDEN (1), Jennifer Ames (1), and Sachin Chandra (2). (1) School of Food Biosciences, The University of Reading, PO Box 226, Reading, RG6 6AP UK, and (2) Brewing Research International, Lyttel Hall, Nutfield, Surrey, RH1 4HY, UK.

The effect of the malting process on the antioxidant activity of pale and speciality malts is currently a very active area of research. However, the contribution of these antioxidants to the beer and the effects of the complete brewing process on changes in antioxidant activity is less well understood. The aim of this study was to determine the effect of each stage of the brewing process for best bitter on the antioxidant activity, color and selected malt flavor compounds. Antioxidant activity was carried out on unfractionated samples, low molecular mass (LMM) (<5 kDa) and high molecular mass (HMM) (>5 kDa) fractions, using the 2,2'-azino-bis(3-ethylbenothiazoline)-6-sulfonic acid radical cation (ABTS (^radical+) scavenging method and ferric reducing antioxidant power (FRAP) assay. Serial dilution color profiles were constructed from CIEL*a*b* tristimulus values, and the fate of selected malt flavor compounds was monitored using gas chromatography-mass spectrometry. Changes in the serial dilution color profile occurred after boiling, fermentation and clarification, with the profile after clarification being the same as that at the end of boiling. The majority of the flavor compounds originating from the malt were lost during brewing, with 3-methylbutanal, 2-methylbutanal, furfural, hexanal and E-2-nonenal being found above their odor threshold levels in the final beer. Both of the antioxidant assays showed that the LMM fraction contributed the most antioxidant activity (75-90%). The most critical stages during the brewing process for changes in antioxidant activity as assessed by both assays were filtration and clarification, with clarification also having a significant effect on the color of the beer. Several of the other stages indicated a change in antioxidant activity as assessed by either the ABTS (^radical+) or FRAP procedure. These included boiling, fermentation, maturation and pasteurisation. Both filtration and clarification technologies warrant further investigation for optimisation of antioxidant activity in beer.

Helen Woffenden received a B.Sc. with First Class Honours in Food Science from the University of Reading, U.K. in 1999. Since 1999, she has been working for her Ph.D. in the School of Food Biosciences at The University of Reading, in collaboration with Brewing Research International, on the characterisation of thermally induced antioxidants during malting and brewing.

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